Personally, I like Backcountry Hunters and Anglers for their work on public land access. That is just my opinion though, I know plenty of people out there that don’t like them as much due to some of their initiatives.
It’s all a matter of reading/knowing the groups policies and how they align with your beleifs.
I’m a member of a few different conservation organizations. The ones that I tend to join are usually pretty close to the game that I hunt (i.e. National Deer Association for Deer Hunting, NWTF for Turkey, etc).
I agree with @Jamesbush in the sense that there isn’t necessarily a “best” one. To me, it’s more about finding a group that matches your values and goals.